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Fabrication of MOF Thin Films at Miscible Liquid-Liquid Interface by Spray Method

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  • 2020-12-10 15:07:03
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FabricationofMOFThinFilmsatMiscibleLiquid−LiquidInterfacebySprayMethodXiao-jueBai,†DanChen,†Lin-linLi,†LeiShao,†Wen-xiuHe,†HuanChen,†Yu-nongLi,†Xue-minZhang,†Li-yingZhang,†Tie-qiangWang,†YuFu,*,†andWeiQi*,‡†DepartmentofChemistry,CollegeofSciences,NortheasternUniversity,Shenyang110819,P.R.China‡ShenyangNationalLaboratoryforMaterialsScience,InstituteofMetalResearch,ChineseAcademyofSciences,Shenyang110016,P.R.China*SSupportingInformationABSTRACT:Metal−organicframeworks(MOFs)areanintriguingclassofporouscrystallineinorganic−organichybridmaterials.Thefabricationoforiented,crystallinethinfilmofMOFsisexpectedtoopennovelavenuestotraditionalapplicationsandtoservemyriadadvancedtechnologies.Here,afacilespray-assistedmiscibleliquid−liquidinterface(MLLI)syntheticstrategyiscarriedoutandreportedundermildconditionthatutilizesmiscibleinterfacefortherapidandcontrollablefabricationoflarge-areafree-standingMOFthinfilms.Themethodologycanemployvariousmetalnodesandorganicligandstoyieldvarioushighqualitylamella

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